Introduction to Ligand Coverage
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In this study, we show that the mechanism of size focusing involves a dependence of the growth rate on the size of the nanoparticles and the ligand coverage on the surface of the nanoparticles.
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Here, the authors use dSTORM imaging and probabilistic modelling to map the distribution of fluorophores on a nanoparticle, finding that ligand coverage is heterogeneous and highly variable between individual particles.
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The decrease in the surface energy increases with ligand coverage.
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We report the results of molecular dynamics simulations of the properties of a pseudo-atom (united atom) model of dodecane thiol ligated 5-nm diameter gold nanoparticles (AuNPs) in a vacuum as a function of ligand coverage and particle separation in three states of aggregation, namely, the isolated AuNPs, the isolated pair of AuNPs, and a square lattice of four AuNPs.
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However, the ligand coverage, which could also tune electronic properties, is always ignored.
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This work is essential for a deeper understanding of the fundamental forces that direct nanocrystal assembly including nanocrystal shape and ligand coverage.
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