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fluorescent supramolecular polymer

We presented the construction of a lead chalcogenide quantum dot-based fluorescent supramolecular polymer network driven by pillar[5]arene-based host–guest complexation.

Formation of a lead chalcogenide quantum dot-based supramolecular polymer network via pillar[5]arene-based host–guest complexation

fluorescent supramolecular polymer

A fluorescent supramolecular polymer network with an excellent triple-stimuli responsive property based on metal–ligand coordination and host–guest interactions has been constructed from a terpyridine-monofunctionalized leaning tower[6]arene, a tetraphenylethylene AIEgen, and a bridging coordination ion (Zn2+).

Stimuli-responsive fluorescent supramolecular polymer network based on a monofunctionalized leaning tower[6]arene

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fluorescent supramolecular system

This study provides insight into construct cationic cage with both fluorescence and host-guest properties, and might facilitate further design of multifunctional cages and other fluorescent supramolecular systems based on host-guest recognition.

Tetraphenylethene-Based Octacationic Cage.

fluorescent supramolecular system

We construct a fluorescent supramolecular system (TPE-Q4⊂ DSP5) of excellent tolerance to a wide range of pH by the facile self-assembly of a new pillar[5]arene bearing disulfonated arms (DSP5) with an AIE-active tetraphenylethene-based tetratopic guest bearing four quaternary ammonium binding sites (TPE-Q4), which exhibits strong blue emission even in dilute aqueous solutions along with much higher quantum yield and longer fluorescence lifetime than TPE-Q4 itself.

A Binary Supramolecular Assembly with Intense Fluorescence Emission, High pH Stability, and Cation Selectivity: Supramolecular Assembly-Induced Emission Materials

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10.1039/d1qm00699a

We presented the construction of a lead chalcogenide quantum dot-based fluorescent supramolecular polymer network driven by pillar[5]arene-based host–guest complexation.

Formation of a lead chalcogenide quantum dot-based supramolecular polymer network via pillar[5]arene-based host–guest complexation

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10.1002/anie.202111213

Herein, we report that the hierarchical self-assembly of tetraphenylethylene (TPE)-featured metal-organic cages (MOCs) and β-cyclodextrin-conjugated polyethylenimine can generate fluorescent supramolecular nanoparticles (FSNPs) to deliver protein into neural cells, a hard-to-transfect cell line using conventional strategy.

Tetraphenylethylene-featured Fluorescent Supramolecular Nanoparticles for Intracellular Trafficking of Protein Delivery and Neuroprotection.

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10.1002/chem.202102296

We report here a set of fluorescent supramolecular organic frameworks (SOFs) that incorporate aggregation-induced emission (AIE) units within their frameworks.

Fluorescent Supramolecular Organic Frameworks Constructed by Amidinium-Carboxylate Salt Bridges.

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10.1002/chem.202005184

In this study, photoswitchable fluorescent supramolecular metallacycles with high fatigue-resistance have been constructed by coordination-driven self-assembly by using bithienylethene with dipyridyl units ( BTE ) as a donor and a fluorescent di-platinum(II) ( Pt-F ) as an acceptor.

Photoswitchable Fluorescent Self-Assembled Metallacycles with High Photostability.

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10.1021/acsami.1c02994

By the combination of various external stimuli, these fluorescent supramolecular host-guest systems could reveal interesting photoluminescence (PL) properties in DMF/H2O (1:1, v/v) solutions, including bifluorophoric host-guest systems after the complexation of Al3+ ion, i.

Controllable FRET Behaviors of Supramolecular Host-Guest Systems as Ratiometric Aluminum Ion Sensors Manipulated by Tetraphenylethylene-Functionalized Macrocyclic Host Donor and Multistimuli-Responsive Fluorescein-Based Guest Acceptor.

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10.1016/J.CCR.2021.213792

This review focuses on the recent development of fluorescent supramolecular gels as sensors for applications in environmental and biological field, in which these fluorescent chemosensors can selectively detect specific metal ions, organic compounds or gases.

Fluorescent supramolecular self-assembly gels and their application as sensors: A review

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10.1039/d1an00218j

A carbon dot (CD) doped fluorescent supramolecular lanthanide coordination polymer (CDs@Tb-GMP) was prepared with Tb3+ and the ligand guanine single nucleotide (GMP).

A carbon dot doped lanthanide coordination polymer nanocomposite as the ratiometric fluorescent probe for the sensitive detection of alkaline phosphatase activity.

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10.1016/J.JPHOTOCHEM.2021.113414

The observed quenching of the fluorescence bands in [M(II)Ln]2+ can be described in terms of a static process mechanism, attributed to a non-fluorescent supramolecular interaction of [M(II)Ln]2+ with C60.

Robust fluorogenic non-porphyrin interaction of Zn(II) and Hg(II) naphthadiaza-crown macrocyclic complexes with C60: Spectroscopic and dispersion-corrected DFT study

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10.1039/c9nr04593g

This work demonstrates an unconventional influence of the functional motif in the condensed state that could emerge as a promising route to build a fluorescent supramolecular nanoassembly from non-fluorescent conjugated molecules for a variety of future applications.

Functional group engineering in naphthalimides: a conceptual insight to fine-tune the supramolecular self-assembly and condensed state luminescence.

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10.1016/j.cclet.2019.10.023

A fluorescent supramolecular polymer network with an excellent triple-stimuli responsive property based on metal–ligand coordination and host–guest interactions has been constructed from a terpyridine-monofunctionalized leaning tower[6]arene, a tetraphenylethylene AIEgen, and a bridging coordination ion (Zn2+).

Stimuli-responsive fluorescent supramolecular polymer network based on a monofunctionalized leaning tower[6]arene

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10.1039/C8PY01396A

These intermolecular noncovalent interactions have been considered to be the main driving forces for fabricating fluorescent supramolecular polymers with AIE properties, and have an important influence on the fluorescence properties of the chromophores.

Fluorescent supramolecular polymers with aggregation induced emission properties

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10.1039/C9TC03243F

A new fluorescent supramolecular self-assembly gelator (1) based on naphthalimide derivative with a tetrazole group was designed and synthesized, which could form a stable gel in acetone/H2O (1/1, v/v).

Multifunctional fluorescent naphthalimide self-assembly system for the detection of Cu2+ and K+ and continuous sensing of organic amines and gaseous acids

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10.1038/s41467-019-12204-7

Fluorescent supramolecular coordination complexes are of interest for chemical sensing and optical devices.

Switchable organoplatinum metallacycles with high quantum yields and tunable fluorescence wavelengths

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10.1016/j.bioorg.2019.03.030

Fluorescence and UV-vis assays indicate a static quenching mechanism with non-fluorescent supramolecular complex formation and changing the native protein structure.

Evaluation of guanylhydrazone derivatives as inhibitors of Candida rugosa digestive lipase: Biological, biophysical, theoretical studies and biotechnological application.

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10.1002/anie.201912730

This study provides insight into construct cationic cage with both fluorescence and host-guest properties, and might facilitate further design of multifunctional cages and other fluorescent supramolecular systems based on host-guest recognition.

Tetraphenylethene-Based Octacationic Cage.

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10.34133/2019/1454562

We construct a fluorescent supramolecular system (TPE-Q4⊂ DSP5) of excellent tolerance to a wide range of pH by the facile self-assembly of a new pillar[5]arene bearing disulfonated arms (DSP5) with an AIE-active tetraphenylethene-based tetratopic guest bearing four quaternary ammonium binding sites (TPE-Q4), which exhibits strong blue emission even in dilute aqueous solutions along with much higher quantum yield and longer fluorescence lifetime than TPE-Q4 itself.

A Binary Supramolecular Assembly with Intense Fluorescence Emission, High pH Stability, and Cation Selectivity: Supramolecular Assembly-Induced Emission Materials

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10.1038/s41598-019-47588-5

Pyrazine derivatives DIPY, TETPY and CNDIPY have been designed and synthesized which form fluorescent supramolecular assemblies in mixed aqueous media due to their AIEE and ICT characteristics.

AIEE Active Nanoassemblies of Pyrazine Based Organic Photosensitizers as Efficient Metal-Free Supramolecular Photoredox Catalytic Systems

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10.1007/s10118-019-2305-1

Furthermore, pH-triggered release of an encapsulated water-insoluble drug (doxorubicin) from the self-assembled fluorescent supramolecular polymersomes is also investigated.

Fluorescent Supramolecular Polymersomes Based on Pillararene/Paraquat Molecular Recognition for pH-controlled Drug Release

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10.1016/J.CCLET.2019.08.027

During the past few years, the construction of fluorescent supramolecular metallocycles has attracted extensive attention due to their diverse applications such as sensing, photoelectric devices, and mimicking complicated natural photo-processes.

Our expedition in the construction of fluorescent supramolecular metallacycles

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10.1021/jacs.9b01546

Herein, through supramolecular host-guest interactions, a fluorescent supramolecular polymer has been facilely constructed from a newly designed [2]biphenyl-extended pillar[6]arene equipped with two thymine sites as arms (H) and a tetraphenylethylene (TPE)-bridged bis(quaternary ammonium) guest (G) with aggregation-induced emission (AIE) property.

Supramolecular Assembly-Induced Emission Enhancement for Efficient Mercury(II) Detection and Removal.

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10.1016/J.SNB.2019.03.112

We show that fluorescent supramolecular biosensors (fSBs) can selectively detect E.

A fluorescent supramolecular biosensor for bacterial detection via binding-induced changes in coiled-coil molecular assembly

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10.1021/jacs.9b02617

Interestingly, AIE-active 2 as a single-molecule-based fluorescent supramolecular platform can encapsulate an organic dye (e.

Aggregation-Induced Emission and Light-Harvesting Function of Tetraphenylethene-Based Tetracationic Dicyclophane.

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Fluorescent Supramolecular
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What is/are Fluorescent Supramolecular?

Fluorescent Supramolecular - We presented the construction of a lead chalcogenide quantum dot-based fluorescent supramolecular polymer network driven by pillar[5]arene-based host–guest complexation. [1] Herein, we report that the hierarchical self-assembly of tetraphenylethylene (TPE)-featured metal-organic cages (MOCs) and β-cyclodextrin-conjugated polyethylenimine can generate fluorescent supramolecular nanoparticles (FSNPs) to deliver protein into neural cells, a hard-to-transfect cell line using conventional strategy. [2] We report here a set of fluorescent supramolecular organic frameworks (SOFs) that incorporate aggregation-induced emission (AIE) units within their frameworks. [3] In this study, photoswitchable fluorescent supramolecular metallacycles with high fatigue-resistance have been constructed by coordination-driven self-assembly by using bithienylethene with dipyridyl units ( BTE ) as a donor and a fluorescent di-platinum(II) ( Pt-F ) as an acceptor. [4] By the combination of various external stimuli, these fluorescent supramolecular host-guest systems could reveal interesting photoluminescence (PL) properties in DMF/H2O (1:1, v/v) solutions, including bifluorophoric host-guest systems after the complexation of Al3+ ion, i. [5] This review focuses on the recent development of fluorescent supramolecular gels as sensors for applications in environmental and biological field, in which these fluorescent chemosensors can selectively detect specific metal ions, organic compounds or gases. [6] A carbon dot (CD) doped fluorescent supramolecular lanthanide coordination polymer (CDs@Tb-GMP) was prepared with Tb3+ and the ligand guanine single nucleotide (GMP). [7] The observed quenching of the fluorescence bands in [M(II)Ln]2+ can be described in terms of a static process mechanism, attributed to a non-fluorescent supramolecular interaction of [M(II)Ln]2+ with C60. [8] This work demonstrates an unconventional influence of the functional motif in the condensed state that could emerge as a promising route to build a fluorescent supramolecular nanoassembly from non-fluorescent conjugated molecules for a variety of future applications. [9] A fluorescent supramolecular polymer network with an excellent triple-stimuli responsive property based on metal–ligand coordination and host–guest interactions has been constructed from a terpyridine-monofunctionalized leaning tower[6]arene, a tetraphenylethylene AIEgen, and a bridging coordination ion (Zn2+). [10] These intermolecular noncovalent interactions have been considered to be the main driving forces for fabricating fluorescent supramolecular polymers with AIE properties, and have an important influence on the fluorescence properties of the chromophores. [11] A new fluorescent supramolecular self-assembly gelator (1) based on naphthalimide derivative with a tetrazole group was designed and synthesized, which could form a stable gel in acetone/H2O (1/1, v/v). [12] Fluorescent supramolecular coordination complexes are of interest for chemical sensing and optical devices. [13] Fluorescence and UV-vis assays indicate a static quenching mechanism with non-fluorescent supramolecular complex formation and changing the native protein structure. [14] This study provides insight into construct cationic cage with both fluorescence and host-guest properties, and might facilitate further design of multifunctional cages and other fluorescent supramolecular systems based on host-guest recognition. [15] We construct a fluorescent supramolecular system (TPE-Q4⊂ DSP5) of excellent tolerance to a wide range of pH by the facile self-assembly of a new pillar[5]arene bearing disulfonated arms (DSP5) with an AIE-active tetraphenylethene-based tetratopic guest bearing four quaternary ammonium binding sites (TPE-Q4), which exhibits strong blue emission even in dilute aqueous solutions along with much higher quantum yield and longer fluorescence lifetime than TPE-Q4 itself. [16] Pyrazine derivatives DIPY, TETPY and CNDIPY have been designed and synthesized which form fluorescent supramolecular assemblies in mixed aqueous media due to their AIEE and ICT characteristics. [17] Furthermore, pH-triggered release of an encapsulated water-insoluble drug (doxorubicin) from the self-assembled fluorescent supramolecular polymersomes is also investigated. [18] During the past few years, the construction of fluorescent supramolecular metallocycles has attracted extensive attention due to their diverse applications such as sensing, photoelectric devices, and mimicking complicated natural photo-processes. [19] Herein, through supramolecular host-guest interactions, a fluorescent supramolecular polymer has been facilely constructed from a newly designed [2]biphenyl-extended pillar[6]arene equipped with two thymine sites as arms (H) and a tetraphenylethylene (TPE)-bridged bis(quaternary ammonium) guest (G) with aggregation-induced emission (AIE) property. [20] We show that fluorescent supramolecular biosensors (fSBs) can selectively detect E. [21] Interestingly, AIE-active 2 as a single-molecule-based fluorescent supramolecular platform can encapsulate an organic dye (e. [22]

fluorescent supramolecular polymer

We presented the construction of a lead chalcogenide quantum dot-based fluorescent supramolecular polymer network driven by pillar[5]arene-based host–guest complexation. [1] A fluorescent supramolecular polymer network with an excellent triple-stimuli responsive property based on metal–ligand coordination and host–guest interactions has been constructed from a terpyridine-monofunctionalized leaning tower[6]arene, a tetraphenylethylene AIEgen, and a bridging coordination ion (Zn2+). [2] These intermolecular noncovalent interactions have been considered to be the main driving forces for fabricating fluorescent supramolecular polymers with AIE properties, and have an important influence on the fluorescence properties of the chromophores. [3] Herein, through supramolecular host-guest interactions, a fluorescent supramolecular polymer has been facilely constructed from a newly designed [2]biphenyl-extended pillar[6]arene equipped with two thymine sites as arms (H) and a tetraphenylethylene (TPE)-bridged bis(quaternary ammonium) guest (G) with aggregation-induced emission (AIE) property. [4]

fluorescent supramolecular system

This study provides insight into construct cationic cage with both fluorescence and host-guest properties, and might facilitate further design of multifunctional cages and other fluorescent supramolecular systems based on host-guest recognition. [1] We construct a fluorescent supramolecular system (TPE-Q4⊂ DSP5) of excellent tolerance to a wide range of pH by the facile self-assembly of a new pillar[5]arene bearing disulfonated arms (DSP5) with an AIE-active tetraphenylethene-based tetratopic guest bearing four quaternary ammonium binding sites (TPE-Q4), which exhibits strong blue emission even in dilute aqueous solutions along with much higher quantum yield and longer fluorescence lifetime than TPE-Q4 itself. [2]