Introduction to Pd Catalyzed Oxidative
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We then report the first Pd-catalyzed oxidative carbonylation in which the oxidant could be completely replaced by visible light.
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Here, we report catalyst-controlled regioselectivity in the Pd-catalyzed oxidative coupling of N-(phenylsulfonyl)indoles and aryl boronic acids using O2 as the oxidant.
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Derived from a Pd-catalyzed oxidative C-H/C-H coupling reaction, two giant imidazole-based [60]tetradecaphyrins adopting stable figure-eight geometry together with one [30]heptaphyrin are obtained by [5 + 2] MacDonald condensations in one pot.
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Herein, we report the synthesis of 3-carbonyl-trisubstituted furans via Pd-catalyzed oxidative cycloisomerization reactions of 2-alkenyl-1,3-dicarbonyl scaffolds, using molecular oxygen as the sole oxidant to regenerate active palladium catalytic species, featuring good functional tolerance and mild reaction conditions.
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However, the achievement of high palladium efficiency and selectivity in Pd-catalyzed oxidative cascade reactions is still challenging in many cases, as a result of the aggregation of active palladium species to Pd black and the possible side reactions during each bond-forming step.
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A variety of functional groups, including ester, amide, ketone, aldehyde, and nitrile, on the heterocyclic cores were tolerated in Pd-catalyzed oxidative reactions.
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This newly introduced ligand class is complementary to the ligands developed for Pd-catalyzed oxidative reactions and may find broad application in transition-metal-catalyzed reactions.
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We report a (thioether)Pd-catalyzed oxidative coupling method for the rapid assembly of both privileged oligothiophenes and challenging hindered cases, even at low catalyst loading under Ag- and Cu-free conditions.
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The reaction represents a segue into the powerful Pd-catalyzed oxidative transformations of organosilanes.
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We demonstrate the use of this approach on the origins of catalyst-controlled anti-Markovnikov-selectivity in Hull's Pd-catalyzed oxidative amination reactions.
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Benzyl and allyltriflamides can engage in Pd-catalyzed oxidative (4+2) annulations with allenes, to produce highly valuable tetrahydroisoquinoline or dihydropyridine skeletons.
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A short and efficient synthetic approach for brivaracetam has been accomplished via two different routes which utilize Pd-catalyzed oxidative cyclization and ring-closing metathesis (RCM) as the key reaction.
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A novel Pd-catalyzed oxidative Heck reaction with readily available Grignard reagents using di- t-butyldiaziridinone as an oxidant has been developed.
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Salient features of the work include a Pd-catalyzed oxidative cyclization to assemble the [3.
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The Pd-catalyzed oxidative Heck coupling reaction proceeds under an oxygen atmosphere at room temperature, in the absence of a base and/or a ligand, showing excellent practicality of the process.
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